Model-free multiparametric analysis of SHG images reveals collagen signatures in breast cancer

Nature作者:Raffaella Mercatelli2026年8月12日正文已收录本站
  • Article
  • Open access
  • Published:
  • Giuseppe Massimo Bernava2,
  • Tiziana Triulzi3,
  • Rosaria Orlandi3,
  • Giuseppe Lombardo2 &
  • …
  • Riccardo Cicchi4,5 

Scientific Reports (2026) Cite this article

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Abstract

We present a novel multiparametric approach for analyzing high-resolution polarization-resolved Second-Harmonic Generation (pSHG) images to identify aligned collagen bundles in histological samples of human breast cancer. This method introduces a model-free optical biomarker—Polarization Asymmetry (PA)—which quantify collagen supramolecular organization without relying on assumed symmetry models. This biomarker was compared with both the angular phase shift (ϕ0) of pSHG intensity curves and the |χyyy| component of the second-order susceptibility tensor, derived from fitting pSHG data to a trigonal symmetry model. Our results reveal that high values of PA, |χyyy|, and ϕ0 variation over micrometric scale, consistently detect the presence of aligned collagen bundles, suggesting a correlation with the structural remodeling of the extracellular matrix at the sub-micrometric scale that may influence tissue mechanical properties. Validation on human corneal tissue, characterized by well-known collagen architecture and biomechanics, confirmed the robustness and generalizability of our approach for detecting diagnostically relevant collagen signatures in cancer and other collagen-rich tissues.

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Acknowledgements

The authors wish to thank Alessandro Ruzza from ‘Fondazione Banca degli occhi del Veneto—Onlus’ for providing corneal tissues.

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Authors and Affiliations

  1. Institute for Biomedical Technologies, CNR-ITB, National Research Council, Via Giuseppe Moruzzi 1, 56124, Pisa, Italy

    Raffaella Mercatelli

  2. CNR-IPCF, Istituto per i Processi Chimico-Fisici, Viale F. Stagno D’Alcontres 37, 98158, Messina, Italy

    Giuseppe Massimo Bernava & Giuseppe Lombardo

  3. Department of Experimental Oncology, Fondazione IRCCS Istituto Nazionale dei Tumori di Milano, Milan, Italy

    Tiziana Triulzi & Rosaria Orlandi

  4. CNR-INO, National Institute of Optics, National Research Council, Largo Enrico Fermi 6, 50125, Florence, Italy

    Riccardo Cicchi

  5. LENS, European Laboratory for Non-linear Spectroscopy, Via Nello Carrara 1, 50019, Sesto Fiorentino, Italy

    Riccardo Cicchi

Authors

  1. Raffaella Mercatelli
  2. Giuseppe Massimo Bernava
  3. Tiziana Triulzi
  4. Rosaria Orlandi
  5. Giuseppe Lombardo
  6. Riccardo Cicchi

Corresponding author

Correspondence to Raffaella Mercatelli.

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The authors declare no competing interests.

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Mercatelli, R., Bernava, G.M., Triulzi, T. et al. Model-free multiparametric analysis of SHG images reveals collagen signatures in breast cancer. Sci Rep (2026). https://doi.org/10.1038/s41598-026-62801-y

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  • DOI: https://doi.org/10.1038/s41598-026-62801-y